Browsing by Author "Chao, K. S."

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Orbital ordering of layered manganites from resonant soft X-ray scattering
(2007-03-01)
Chao, K. S.
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Huang, D. J.
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Okamoto, J.
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Lin, H.-J.
;
Hsu, C.-H.
We present measurements of Mn L-edge resonant soft X-ray scattering on single-layered manganites with different sizes of cations. Orbital ordering of Pr0.5Ca1.5MnO4 exhibits a stronger three-dimensional character and a dramatically enhanced transition temperature, as compared with those of La0.5Sr1.5MnO4. The c-axis correlation length of orbital ordering in Pr0.5Ca1.5MnO4 is about half of the inplane correlation length. Our results indicate that reduction in one-electron bandwidth and quenched disorder strongly enhances the stabilization of charge-orbital ordering. (c) 2006 Published by Elsevier B. V.
Quasi-two-dimensional d-spin and p-hole ordering in the three-dimensional perovskite La(1/3)Sr(2/3)FeO(3)
(2010-10-22)
Okamoto, J.
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Huang, D. J.
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Chao, K. S.
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Huang, S. W.
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Hsu, C. -H.
Measurements of resonant soft x-ray magnetic scattering reveal anomalous ordering of 3d spins and 2p holes in perovskite La(1/3)Sr(2/3)FeO(3), which is known to exhibit three-dimensional (3D) charge and spin ordering along the (111) direction. Upon cooling, a quasi-two-dimensional phase consisting of ferromagnetic and charge-disproportionated [111] trilayers of Fe(3+)-Fe(5+)-Fe(3+) precedes the development of 3D magnetic ordering at the transition temperature, in sharp contrast to an ordinary transition from the paramagnetic and charge-uniform phase to the antiferromagnetic and charge-disproportionated phase expected according to conventional wisdom.
Quasi-two-dimensional d-spin and p-hole ordering in the three-dimensional perovskite La1/3Sr2/3FeO3
(2010-10-22)
Okamoto, J.
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Huang, D. J.
;
Chao, K. S.
;
Huang, S. W.
;
Hsu, C. -H.
Measurements of resonant soft x-ray magnetic scattering reveal anomalous ordering of 3d spins and 2p holes in perovskite La1/3Sr2/3FeO3, which is known to exhibit three-dimensional (3D) charge and spin ordering along the (111) direction. Upon cooling, a quasi-two-dimensional phase consisting of ferromagnetic and charge-disproportionated [111] trilayers of Fe3+-Fe5+-Fe3+ precedes the development of 3D magnetic ordering at the transition temperature, in sharp contrast to an ordinary transition from the paramagnetic and charge-uniform phase to the antiferromagnetic and charge-disproportionated phase expected according to conventional wisdom.
Symmetry of multiferroicity in a frustrated magnet TbMn2O5
(2007-04-13)
Okamoto, J.
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Huang, D. J.
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Mou, C. -Y.
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Chao, K. S.
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Lin, H. -J.
Based on measurements of soft-x-ray magnetic scattering and symmetry considerations, we demonstrate that the magnetoelectric effect in TbMn2O5 arises from an internal field determined by (S) over right arrow ((q) over right arrow) x (s) over right arrow (-(q) over right arrow) with (S) over right arrow ((q) over right arrow) being the magnetization at modulation vector (q) over right arrow, whereas the magnetoelastic effect in the exchange energy governs the response to external electric fields. Our results set fundamental symmetry constraints on the microscopic mechanism of multiferroicity in frustrated magnets.
Thermally or Magnetically Induced Polarization Reversal in the Multiferroic CoCr(2)O(4)
(2009-02-13)
Choi, Y. J.
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Okamoto, J.
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Huang, D. J.
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Chao, K. S.
;
Lin, H. J.
We report the unexpected evolution, with thermal and magnetic-field (H) variations, of the interrelation between the polarization P, magnetization M, and spiral wave vector Q in CoCr(2)O(4), which has a ferrimagnetic conical-spiral magnetic order. For example, P suddenly jumps and changes its sign at the magnetic lock-in transition (T(L)) with thermal variation, or with isothermal variation of H (without changing its direction) at T(L), which surprisingly occurs without change in spiral handedness (i.e., the sign of Q). The presence of multiple spiral sublattices may be behind this unusual behavior.
Thermally or Magnetically Induced Polarization Reversal in the Multiferroic CoCr2O4
(2009-02-13)
Choi, Y. J.
;
Okamoto, J.
;
Huang, D. J.
;
Chao, K. S.
;
Lin, H. J.
We report the unexpected evolution, with thermal and magnetic-field (H) variations, of the interrelation between the polarization P, magnetization M, and spiral wave vector Q in CoCr2O4, which has a ferrimagnetic conical-spiral magnetic order. For example, P suddenly jumps and changes its sign at the magnetic lock-in transition (T-L) with thermal variation, or with isothermal variation of H (without changing its direction) at T-L, which surprisingly occurs without change in spiral handedness (i.e., the sign of Q). The presence of multiple spiral sublattices may be behind this unusual behavior.