Browsing by Author "Cheng, P. C."

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3D visualizations of nanoscale phase separation and ultrafast dynamic correlation between phases in (Na0.32K0.68)(0.95)Fe1.75Se2
(2019-03-25)
Cheng, P. C.
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Tzeng, W. Y.
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Chu, Y. J.
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Luo, C. W.
;
Zhukov, A. A.
Phase separation of metallic and antiferromagnetic (AFM) insulating phases in alkaline iron selenides (A(x)Fe(2)-ySe(2)) continues to attract intense interest because the relationship between two peculiar features probably is a key to clarifying the pairing mechanism of A(x)Fe(2-y)Se(2) superconductors. Here we report that the three-dimensional (3D) visualizations of nanoscale phase separation in (Na0.32K0.68)(0.95)Fe1.75Se2 single crystals are revealed by hybrid focused-ion-beam scanning electron microscopy and the superconducting paths are fully percolative in 3D. Moreover, the phase-related ultrafast dynamics in (Na0.32K0.68)(0.95)Fe1.75Se2 is studied by dual-color pump-probe spectroscopy. The anomalous changes in the electron and acoustic phonon components of transient reflectivity change (Delta R/R) identify two characteristic temperatures T* similar to 100K (the onset temperature of coupling between the nanometallic and AFM phases) and T-H similar to 230K (the onset temperature of the metallic-interface phase). An energy-transfer channel between the nanometallic and AFM phases is inferred. This proposed channel provides insight into the pairing mechanism of alkaline iron selenide superconductors.
Dynamics of phonons in Sr3Ir4Sn13: an experimental study by ultrafast spectroscopy measurements
(2016-07-26)
Luo, C. W.
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Cheng, P. C.
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Tu, C. M.
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Kuo, C. N.
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Wang, C. M.
We report a study of ultrafast dynamics of photoexcited electrons and phonons in Sr3Ir4Sn13 using dual-color transient reflectivity change (Delta R/R) measurements. Time resolved optical spectroscopy of collective excitations reveal the marked features near its structural phase transition temperature T* similar or equal to 147 K. Two distinctive oscillatory timescales in Delta R/R have been clearly resolved. The rapid THz-range oscillations are attributed to the dynamics of the optical phonons which strongly correlate to the structural phase transition. The slow GHz-range oscillatory phenomenon which only occurs below about 150 K is associated with the dynamic response of the longitudinal-acoustic phonons. These low-energy phonons show a softening feature on approaching the transition temperature, also indicating a strong relevance to the structural phase transition. The information that we demonstrated would provide a deeper understanding of the structural phase transition in Sr3Ir4Sn13.
Fabrication and characteristics of thin-film InGaN-GaN light-emitting diodes with TiO2/SiO2 omnidirectional reflectors
(2007-07-01)
Chiu, C. H.
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Kuo, H. C.
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Lee, C. E.
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Lin, C. H.
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Cheng, P. C.
In this paper, a novel GaN-based thin-film vertical injection light-emitting diode (LED) structure with a TiO2 and SiO2 omnidirectional reflector (ODR) and an n-GaN rough surface is designed and fabricated. The designed ODR, consisting of alternating TiO2 and SiO2, layers possesses a complete photonic band gap within the blue region of interest. The arrays of the conducting channels are integrated into the TiO2/SiO2 ODR structure for vertically spreading the current. Assisted by the laser lift-off and photo-enhanced chemically etched surface roughening process, the light output power and the external quantum efficiency of our thin-film LED with a TiO2/SiO2 ODR (at a driving current of 350 mA and with chip size of 1 mm x 1 mm) reached 330 mW and 26.7%, increased by 18% and 16%, respectively, compared with the results from the thin-film LED with an Al mirror. By examining the radiation patterns of the LEDs, the optical output power mainly increased within the 120 deg cone due to the higher reflectance of the TiO2/SiO2 ODR within the blue regime.
Quasiparticle Dynamics and Phonon Softening in FeSe Superconductors
(2012-06-20)
Luo, C. W.
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Wu, I. H.
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Cheng, P. C.
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Lin, J. -Y.
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Wu, K. H.
Quasiparticle dynamics of FeSe single crystals revealed by dual-color transient reflectivity measurements (Delta R/R) provides unprecedented information on Fe-based superconductors. The amplitude of the fast component in Delta R/R clearly gives a competing scenario between spin fluctuations and superconductivity. Together with the transport measurements, the relaxation time analysis further exhibits anomalous changes at 90 and 230 K. The former manifests a structure phase transition as well as the associated phonon softening. The latter suggests a previously overlooked phase transition or crossover in FeSe. The electron-phonon coupling constant lambda is found to be 0.16, identical to the value of theoretical calculations. Such a small lambda demonstrates an unconventional origin of superconductivity in FeSe.
Quasiparticle Dynamics in FeSe Superconductors Studied by Femtosecond Spectroscopy
(2013-04-01)
Luo, C. W.
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Wu, I. H.
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Cheng, P. C.
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Lin, J. -Y.
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Wu, K. H.
The ultrafast quasiparticle dynamics in FeSe single crystals were measured by using dual-color transient reflectivity measurements (Delta R/R) from 4.4 to 290 K. In general, the typical Delta R/R of FeSe includes two significant components. One is the relaxation of photoinduced quasiparticles, which has been used to estimate the electron-phonon coupling strength (lambda=0.16). The other is the oscillation component due to the acoustic phonon. Moreover, the acoustic phonon's energy estimated from the period of oscillation in Delta R/R markedly shrinks around 90 K, which is the so-called phonon softening.
Ultrafast dynamics and phonon softening in Fe1+ySe1-xTex single crystals
(2012-10-31)
Luo, C. W.
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Wu, I. H.
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Cheng, P. C.
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Lin, J-Y
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Wu, K. H.
The ultrafast quasiparticle dynamics of Fe1+ySe1-xTex single crystals were investigated by dual-color transient reflectivity measurements (Delta R/R) from 4.3 to 290 K. The electron-phonon coupling strength lambda (= 0.16-0.01) and the temperature-dependent energy of longitudinal-acoustic phonons were, respectively, obtained from the relaxation time of a fast component and the period of an oscillation component in Delta R/R. Such a small lambda demonstrates the unconventional origin of superconductivity in FeSe. Moreover, the temperature-dependent Delta R/R exhibits anomalous changes at T-c, 90 K and 230 K, unambiguously revealing the phase transition as well as the phonon softening via the magnetoelastic effect.