Browsing by Author "Haung, Jing-Yu"

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Coherent and Polarized Random Laser Emissions from Colloidal CdSe/ZnS Quantum Dots Plasmonically Coupled to Ellipsoidal Ag Nanoparticles
(2017-02)
Yao, Yung-Chi
;
Yang, Zu-Po
;
Hwang, Jung-Min
;
Su, Hai-Ching
;
Haung, Jing-Yu
This study demonstrates the capability of controlling optical anisotropy of lasing emissions by manipulating the coupling strength spatially and spectrally between the oscillated electric field of emitted light and the localized surface plasmon (LSP) resonance for a random lasing medium composed of colloidal CdSe/ZnS quantum dots (QDs) and ellipsoidal silver nanoparticles (Ag NPs). Distinctive from the amplified spontaneous emission generally observed on colloidal CdSe/ZnS QDs, it has been found that lasing emissions of the revealed system exhibit clear interference features (coherent optical feedbacks) with low-threshold characteristics, mainly attributed to enhanced light scatterings and optical gains arisen in peripheral surfaces of ellipsoidal Ag NPs. Importantly, the relative orientation, between the oscillated electric field of emitted light from colloidal CdSe/ZnS QDs and the ellipse axis of Ag NPs, plays a critical role in selective excitation of LSP resonances leading to laser emissions with preferential optical polarizations. The achievement of spatial and spectral coupling of LSP resonance with colloidal QDs, respectively, by spin coating thin QDs film on Ag NPs and control of the Ag NP geometry makes the present system one of the promising candidates of colloidal QDs-based random lasers to achieve coherent and polarized lasing emissions.
Enhanced external quantum efficiency in GaN-based vertical-type light-emitting diodes by localized surface plasmons
(2016-03-03)
Yao, Yung-Chi
;
Hwang, Jung-Min
;
Yang, Zu-Po
;
Haung, Jing-Yu
;
Lin, Chia-Ching
Enhancement of the external quantum efficiency of a GaN-based vertical-type light emitting diode (VLED) through the coupling of localized surface plasmon (LSP) resonance with the wave-guided mode light is studied. To achieve this experimentally, Ag nanoparticles (NPs), as the LSP resonant source, are drop-casted on the most top layer of waveguide channel, which is composed of hydrothermally synthesized ZnO nanorods capped on the top of GaN-based VLED. Enhanced light-output power and external quantum efficiency are observed, and the amount of enhancement remains steady with the increase of the injected currents. To understand the observations theoretically, the absorption spectra and the electric field distributions of the VLED with and without Ag NPs decorated on ZnO NRs are determined using the finite-difference time-domain (FDTD) method. The results prove that the observation of enhancement of the external quantum efficiency can be attributed to the creation of an extra escape channel for trapped light due to the coupling of the LSP with wave-guided mode light, by which the energy of wave-guided mode light can be transferred to the efficient light scattering center of the LSP.
Enhancing UV-emissions through optical and electronic dual-function tuning of Ag nanoparticles hybridized with n-ZnO nanorods/p-GaN heterojunction light-emitting diodes
(2016)
Yao, Yung-Chi
;
Yang, Zu-Po
;
Hwang, Jung-Min
;
Chuang, Yi-Lun
;
Lin, Chia-Ching
ZnO nanorods (NRs) and Ag nanoparticles (NPs) are known to enhance the luminescence of light-emitting diodes (LEDs) through the high directionality of waveguide mode transmission and efficient energy transfer of localized surface plasmon (LSP) resonances, respectively. In this work, we have demonstrated Ag NP-incorporated n-ZnO NRs/p-GaN heterojunctions by facilely hydrothermally growing ZnO NRs on Ag NP-covered GaN, in which the Ag NPs were introduced and randomly distributed on the p-GaN surface to excite the LSP resonances. Compared with the reference LED, the light-output power of the near-band-edge (NBE) emission (ZnO, lambda = 380 nm) of our hybridized structure is increased almost 1.5-2 times and can be further modified in a controlled manner by varying the surface morphology of the surrounding medium of the Ag NPs. The improved light-output power is mainly attributed to the LSP resonance between the NBE emission of ZnO NRs and LSPs in Ag NPs. We also observed different behaviors in the electroluminescence (EL) spectra as the injection current increases for the treatment and reference LEDs. This observation might be attributed to the modification of the energy band diagram for introducing Ag NPs at the interface between n-ZnO NRs and p-GaN. Our results pave the way for developing advanced nano-structured LED devices with high luminescence efficiency in the UV emission regime.
Plasmonically Induced Coherent and Polarized Random Laser Emissions in Colloidal CdSe/ZnS Quantum Dots with Ellipsoidal Ag Nanoparticles
(2017-01-01)
Yao, Yung-Chi
;
Yang, Zu-Po
;
Haung, Jing-Yu
;
Lee, Min-Hung
;
Lee, Ya-Ju
We demonstrate the capability of controlling the optical anisotropy of lasing emissions by manipulating the coupling between the oscillated electric field and the localized surface plasmon (LSP) resonance for a random lasing medium composed of colloidal CdSe/ZnS quantum dots (QDs) and ellipsoidal silver nanoparticles (Ag NPs). Distinctive from the amplified spontaneous emission (ASE) generally observed on the CdSe/ZnS QDs, it has been found that lasing emissions of the revealed system exhibit clear interference features with low-threshold characteristics, mainly attributed to enhanced light scatterings and optical gains arisen in the peripheral surfaces of ellipsoidal Ag NPs. Importantly, the relative orientation, between the oscillated electric field of emitted light from CdSe/ZnS QDs and the ellipse axis of Ag NPs, plays a critical role in selective excitation of LSP resonances leading to the laser emissions with preferential optical polarizations. That is further examined and validated by the finite-difference time-domain simulation. The achievement of spatial and spectral coupling of LSP resonance with colloidal QDs respectively make the present system one of the promising candidates of colloidal QDs-based random lasers to achieve coherent and polarized lasing emissions.