Browsing by Author "Hsu, Chu-Yuan"

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Engineering radiative coupling of excitons in 2D semiconductors
(2019-11-20)
Horng, Jason
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Chou, Yu-Hsun
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Chang, Tsu-Chi
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Hsu, Chu-Yuan
;
Lu, Tien-Chang
The resonance energy and the transition rate of atoms, molecules, and solids were understood as their intrinsic properties in classical electromagnetism. It was later realized that these quantities are linked to the radiative coupling between the transition dipole and photon modes. Such effects can be greatly amplified in macroscopic many-body systems from virtual photon exchange between dipoles, but are often masked by inhomogeneity and pure dephasing, especially in solids. Here, we observe in both absorption and emission spectroscopy the renormalization of the exciton resonance and the radiative decay rate in transition metal dichalcogenides monolayers due to their radiative interactions. Tuning the photon mode density near the monolayer, we demonstrate control of cooperative Lamb shift, radiative decay, and valley polarization of the excitons as well as control of the charged exciton emission. Our work establishes a technologically accessible and robust experimental system for engineering cooperative matter-light interactions. (c) 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
Full-Spectrum Analysis of Perovskite-Based Surface Plasmon Nanolasers
(2020-03-29)
Cheng, Pi-Ju
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Zheng, Qi-Yan
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Hsu, Chu-Yuan
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Li, Heng
;
Hong, Kuo-Bin
We systematically studied the characteristics of hybrid perovskite-based surface plasmon nanolasers. If one changes the anion composition of perovskites, the emission wavelength can be easily tuned. We conducted in full-spectrum modeling that featured hybrid perovskite nanowires placed on different SiO2-coated metallic (Au, Ag, and Al) plates. The proposed nanocavities that supported plasmonic gap modes exhibited distinguished properties of nanolasers, such as low-transparency threshold-gain and low lasing threshold. The corresponding experimental results for the MAPbBr(3) nanolaser on Ag revealed the low-threshold operation. These superior features were attributed to enhanced light-matter interaction with strong coupling. Therefore, the proposed scheme, integrated with hybrid perovskite as gain material, provides an excellent platform for nanoscale plasmon lasing in the visible to near-infrared spectra.
Perfect Absorption by an Atomically Thin Crystal
(2020-08-05)
Horng, Jason
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Martin, Eric W.
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Chou, Yu-Hsun
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Courtade, Emmanuel
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Chang, Tsu-chi
Optical absorption is one of the most fundamental processes in light-matter interactions. The ability to achieve and control high absorption is crucial for a broad range of modern photonic technologies. In nanomaterials of length scales much smaller than a wavelength, optical absorption is typically a weak perturbation. To achieve high absorption, exquisite techniques and structures have been developed, such as coherent interference of multiple laser beams and plasmonic metasurfaces. Here, we show that a robust critical-coupling condition exists to allow perfect absorption of light by a subnanometer-thick two-dimensional semiconductor, when the radiative-decay rate of the exciton resonance balances with its loss rate. We measure an absorption up to 99.6% in a monomolecular MoSe2 crystal placed in front of a flat mirror. We furthermore demonstrate control of the perfect absorption by tuning the exciton-phonon, exciton-exciton, and exciton-photon interactions with temperature, pulsed laser excitation, and a movable mirror, respectively. Our work suggests a mechanism to achieve and control critical coupling in two-dimensional excitonic systems, enabling photonic applications including ultrafast low-power light modulators and sensitive optical sensing.
Plasmonic nanolasers based on graphene-insulator-metal platform
(2019-01-01)
Li, Heng
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Hong, Kuo-Bin
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Hsu, Chu-Yuan
;
Huang, Zhen-Ting
;
Lu, Tien-Chang
As the development of nanoscale optics, the ability of surface plasmons to break the diffraction limit receives numerous attention from researchers. In this work, we demonstrate a graphene-insulator-metal (GIM) nanolaser structure. The graphene can modify the permittivity of metal films which would further influence the nanolasers characteristics.
Plasmonic Nanolasers Enhanced by Hybrid Graphene-Insulator-Metal Structures
(2019-08-01)
Li, Heng
;
Li, Jhu-Hong
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Hong, Kuo-Bin
;
Yu, Min-Wen
;
Chun, Yi-Cheng
Graphene is a two-dimensional (2D) structure that creates a linear relationship between energy and momentum that not only forms massless Dirac fermions with extremely high group velocity but also exhibits a broadband transmission from 300 to 2500 nm that can be applied to many optoelectronic applications, such as solar cells, light-emitting devices, touchscreens, ultrafast photodetectors, and lasers. Although the plasmonic resonance of graphene occurs in the terahertz band, graphene can be combined with a noble metal to provide a versatile platform for supporting surface plasmon waves. In this study, we propose a hybrid graphene-insulator-metal (GIM) structure that can modulate the surface plasmon polariton (SPP) dispersion characteristics and thus influence the performance of plasmonic nanolasers. Compared with values obtained when graphene is not used on an Al template, the propagation length of SPP waves can be increased 2-fold, and the threshold of nanolasers is reduced by 50% when graphene is incorporated on the template. The GIM structure can be further applied in the future to realize electrical control or electrical injection of plasmonic devices through graphene.