Browsing by Author "Lai, TL"
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Item type:Item, Quantum dynamics of a diatomic molecule under chirped laser pulses(1998-02-28) ;Lin, JT ;Lai, TL ;Chuu, DS ;Jiang, TF電子物理學系The photodissociation probability of a diatomic molecule is usually very small even under a strong field due to its anharmonicity. However, the progress in laser technology provides a chirped laser pulse to lower the threshold of the dissociation intensity. We investigate the quantum dynamics of a diatomic molecule under such a kind of pulse. It is found that there is a significant dissociation probability at moderate intensity for a diatomic molecule under a chirped pulse. The quantum dissociation probability is found to be suppressed with respect to the classical one for intensities above the dissociation threshold. Therefore the chirped pulse can efficiently dissociate a diatomic molecule.