Browsing by Author "Liu, Tzu-Ming"

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Observation of spontaneous polarization misalignments in periodically poled crystals using second-harmonic generation microscopy
(2011-06-06)
Tzeng, Yu-Yi
;
Zhuo, Zong-Yan
;
Lee, Ming-Yin
;
Liao, Chien-Sheng
;
Wu, Pei-Chun
Periodically poled crystal (PPC) is a key component for nonlinear optical applications. Its poling quality relies largely on successful domain inversion and the alignment of spontaneous polarization (SP) vectors in each domain. Here we report the unexpected observation of bulk second harmonic generation (SHG) in PPC when excitation propagating along its optical axis. Based on its tensorial nature, SHG is highly sensitive to the orientation of SP, and therefore the misalignment of SP in each domain of PPC can be revealed noninvasively by SHG microscopy. This nonlinear imaging modality provides optical sectioning capability with 3D sub-micrometer resolution, so it will be useful for in situ investigation of poling quality in PPC. (C) 2011 Optical Society of America
Resonance-enhanced dipolar interaction between terahertz photons and confined acoustic phonons in nanocrystals
(2008-03-03)
Liu, Tzu-Ming
;
Lu, Ja-Yu
;
Chen, Hung-Ping
;
Kuo, Chung-Chiu
;
Yang, Meng-Ju
Taking advantage of the specific core-shell charge separation structure in the CdSe/CdTe core-shell type-II nanocrystals, we experimentally observed and verified the existence of the resonance-enhanced dipolar interaction between terahertz photons and their corresponding confined acoustic phonons. From the measured terahertz transmission spectra, we found that the photon frequency of the terahertz resonant absorption is inversely proportional to the diameter D of the nanocrystals and agrees with that of dipolar active l=1, n=0 confined acoustic modes. The corresponding absorption cross section shows a D(4) dependence, supporting a charged simple-harmonic-oscillator model. These facts verify the occurrence of dipolar interaction between terahertz photons and confined terahertz acoustic phonons. (c) 2008 American Institute of Physics.
Resonant-Enhanced Dipolar Interaction between THz-Photons and Confined Acoustic Phonons in Nanocrystals
(2008)
Liu, Tzu-Ming
;
Lu, Ja-Yu
;
Chen, Hung-Ping
;
Kuo, Chung-Chiu
;
Lai, Chih-Wei
We proved the existence of resonant-enhanced dipolar interaction between THz-photons and confined acoustic phonons in nanocrystals. By a specific core-shell charge separation, the dipolar (l=1) confined acoustic modes was activated to absorb THz waves. (C) 2007 Optical Society of America
Resonant-enhanced dipolar interaction between THz-photons and confined acoustic phonons in nanostructures
(2008-01-01)
Liu, Tzu-Ming
;
Lu, Ja-Yu
;
Kuo, Chung-Chiu
;
Yang, Meng-Ju
;
Lai, Chih-Wei
By using a frequency-controlled narrow band THz source, a Fourier Transform Infrared (FTIR) spectroscopy system, and a frequency-controlled terahertz (THz) emitter, for the first time, we studied the THz photon absorption related to the THz confined acoustic vibrations in semiconductor nanocrystals. Through a specific charge separation in the CdSe/CdTe type-II nanocrystals and a piezoelectric coupling in the wurtzite CdSe nanocrystals, the THz photons can be resonantly coupled with (l=1) dipolar modes and the (l=0) breathing modes, respectively. Our results provide new mechanisms for low dimensional systems to convert a THz photon into a phonon of the same frequency.