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Now showing 1 - 10 of 18

Perfect Absorption by an Atomically Thin Crystal
(2020-08-05)
Horng, Jason
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Martin, Eric W.
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Chou, Yu-Hsun
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Courtade, Emmanuel
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Chang, Tsu-chi
Optical absorption is one of the most fundamental processes in light-matter interactions. The ability to achieve and control high absorption is crucial for a broad range of modern photonic technologies. In nanomaterials of length scales much smaller than a wavelength, optical absorption is typically a weak perturbation. To achieve high absorption, exquisite techniques and structures have been developed, such as coherent interference of multiple laser beams and plasmonic metasurfaces. Here, we show that a robust critical-coupling condition exists to allow perfect absorption of light by a subnanometer-thick two-dimensional semiconductor, when the radiative-decay rate of the exciton resonance balances with its loss rate. We measure an absorption up to 99.6% in a monomolecular MoSe2 crystal placed in front of a flat mirror. We furthermore demonstrate control of the perfect absorption by tuning the exciton-phonon, exciton-exciton, and exciton-photon interactions with temperature, pulsed laser excitation, and a movable mirror, respectively. Our work suggests a mechanism to achieve and control critical coupling in two-dimensional excitonic systems, enabling photonic applications including ultrafast low-power light modulators and sensitive optical sensing.
Engineering radiative coupling of excitons in 2D semiconductors
(2019-11-20)
Horng, Jason
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Chou, Yu-Hsun
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Chang, Tsu-Chi
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Hsu, Chu-Yuan
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Lu, Tien-Chang
The resonance energy and the transition rate of atoms, molecules, and solids were understood as their intrinsic properties in classical electromagnetism. It was later realized that these quantities are linked to the radiative coupling between the transition dipole and photon modes. Such effects can be greatly amplified in macroscopic many-body systems from virtual photon exchange between dipoles, but are often masked by inhomogeneity and pure dephasing, especially in solids. Here, we observe in both absorption and emission spectroscopy the renormalization of the exciton resonance and the radiative decay rate in transition metal dichalcogenides monolayers due to their radiative interactions. Tuning the photon mode density near the monolayer, we demonstrate control of cooperative Lamb shift, radiative decay, and valley polarization of the excitons as well as control of the charged exciton emission. Our work establishes a technologically accessible and robust experimental system for engineering cooperative matter-light interactions. (c) 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
Fabrication and characteristics of a GaN-based microcavity laser with shallow etched mesa
(2014-06-01)
Lai, Ying-Yu
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Chou, Yu-Hsun
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Wu, Yu-Sheng
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Lan, Yu-Pin
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Lu, Tien-Chang
In this work, we have developed a simple GaN-based microcavity (MC) with an intracavity shallow etched mesa. The textured GaN-based MC incorporated two high-reflectivity dielectric Bragg mirrors and an InGaN/GaN multiple quantum well with a shallow etched mesa as an optical confined structure. Lasing and transverse optical confinement characteristics have been verified by measuring devices with different mesa diameters. A quality factor (Q) of 2600 and a threshold energy of 30 nJ have been observed in a 10-mu m-diameter device. Such a cavity structure could be implanted into electrically pumped GaN vertical-cavity surface-emitting lasers for supporting efficient transverse confinement. (C) 2014 The Japan Society of Applied Physics
High-Performance Plasmonic Nanolasers with a Nanotrench Defect Cavity for Sensing Applications
(2018-07-01)
Cheng, Pi-Ju
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Huang, Zhen-Ting
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Li, Jhu-Hong
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Chou, Bo-Tsun
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Chou, Yu-Hsun
Recent developments in small footprint plasmonic nanolasers show promise for active optical sensing with potential applications in various fields, including real-time and label-free biochemical sensing, and gas detection. In this study, we demonstrate a novel hybrid plasmonic crystal nanolaser that features a ZnO nanowire placed on Al grating surfaces with a nanotrench defect nanocavity. The lasing action of gain-assisted defect nanocavity overcomes the ohmic loss parasitically in the plasmonic nanostructures. Therefore, the plasmonic nanolaser exhibits an extremely small mode volume, a narrow linewidth Delta lambda, and a high Purcell factor that can facilitate the strong interaction between light and matter. This can be used as a refractive index sensor and is highly sensitive to local changes in the refractive indices of ambient materials. By careful design, the near-ultraviolet nanolaser sensors have significant sensing performances of glucose solutions, revealing a high sensitivity of 249 nm/RIU and high resolution, with a figure of merit of 1132, at the resonant wavelength of 373 nm.
Surface plasmon polariton nanolasers: Coherent light sources for new applications
(2018-11-01)
Chou, Yu-Hsun
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Chang, Chia-Jui
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Lin, Tzy-Rong
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Lu, Tien-Chang
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光電工程學系
The invention of the Internet and mobile devices has caused tremendous changes in human lives over the past two decades. Information technology has broken through limitations of geospatial space, enabling extremely high-speed data transmission and new types of data services. In recent years, demands for data processing have shown an increasing trend. Furthermore, data generated from internet-related applications such as cloud services and self-driving technology are likely to grow exponentially over the coming years. Currently, data transmission inside integrated circuits mainly relies on metal wires. However, the substantial resistive-capacitive delay and energy loss that are caused by metal wires limit data transmission speeds. Optical interconnection has been regarded as a major solution to efficiently reduce energy consumption and increase data transmission speeds. The size of conventional semiconductor laser devices, which are the key component in optical interconnection, cannot be smaller than the wavelength of light, which is a fundamental physical obstacle to lasers integrating with current electronic integrated circuits in reasonable volumes. To realize optical interconnection, the volume of the laser device must match the existing electronic components. Recently, the use of diffraction-unlimited plasmonic lasers has been successfully demonstrated, and these have great potential in different applications. In this paper, we discuss the recent progress toward surface plasmon polariton lasers and provide practical insights into the challenges in realizing these novel devices.
Tuning the Characteristics of Surface Plasmon Polariton Nanolasers by Tailoring the Dispersion Relation
(2017-01-01)
Lu, Tien-Chang
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Chou, Yu-Hsun
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Hong, Kuo-Bin
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Chung, Yi-Cheng
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Lin, Tzy-Rong
Nanolasers with ultra-compact footprint are able to provide high intensity coherent light, which have various potential applications in high capacity signal processing, biosensing, and sub-wavelength imaging. Among various nanolasers, those lasers with cavities surrounded with metals have shown to have superior light emission properties due to the surface plasmon effect providing better field confinement capability and allowing exotic light-matter interaction. In this talk, we report robust ultraviolet ZnO nanolaser by using silver (Ag) [1] and aluminum (Al) [2] to strongly shrink the mode volume. The nanolasers operated at room temperature and even high temperature (353K) shows several distinct features including an extremely small mode volume, large Purcell factor and group index. Comparison of characteristics between Ag-and Al-based will also be made.
Metal for Plasmonic Ultraviolet Laser: Al or Ag?
(2017-11-01)
Chou, Yu-Hsun
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Hong, Kuo-Bin
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Chung, Yi-Cheng
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Chang, Chun-Tse
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Chou, Bo-Tsun
Surface plasmon polariton (SPP) nanolasers have recently emerged as promising candidates for generating a coherent light source in nanophotonic integration circuits. The properties of SPP nanolasers, such as group velocity, mode area, modulation speed, and threshold performance, can be manipulated using a dispersion relation. In this study, we investigated the characteristics of SPP nanolasers operated near and far from the SP frequency. Our results indicated that SPP nanolaser performance can be significantly influenced by manipulating the dispersion relation.
Ultracompact Pseudowedge Plasmonic Lasers and Laser Arrays
(2018-02-01)
Chou, Yu-Hsun
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Hong, Kuo-Bin
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Chang, Chun-Tse
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Chang, Tsu-Chi
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Huang, Zhen-Ting
Concentrating light at the deep subwavelength scale by utilizing plasmonic effects has been reported in various optoelectronic devices with intriguing phenomena and functionality. Plasmonic waveguides with a planar structure exhibit a two-dimensional degree of freedom for the surface plasmon; the degree of freedom can be further reduced by utilizing metallic nanostructures or nanoparticles for surface plasmon resonance. Reduction leads to different lightwave confinement capabilities, which can be utilized to construct plasmonic nanolaser cavities. However, most theoretical and experimental research efforts have focused on planar surface plasmon polariton (SPP) nanolasers. In this study, we combined nanometallic structures intersecting with ZnO nanowires and realized the first laser emission based on pseudowedge SPP waveguides. Relative to current plasmonic nanolasers, the pseudowedge plasmonic lasers reported in our study exhibit extremely small mode volumes, high group indices, high spontaneous emission factors, and high Purell factors beneficial for the strong interaction between light and matter. Furthermore, we demonstrated that compact plasmonic laser arrays can be constructed, which could benefit integrated plasmonic circuits.
Controllable lasing performance in solution-processed organic-inorganic hybrid perovskites
(2016)
Kao, Tsung Sheng
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Chou, Yu-Hsun
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Hong, Kuo-Bin
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Huang, Jiong-Fu
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Chou, Chun-Hsien
Solution-processed organic-inorganic perovskites are fascinating due to their remarkable photo-conversion efficiency and great potential in the cost-effective, versatile and large-scale manufacturing of opto-electronic devices. In this paper, we demonstrate that the perovskite nanocrystal sizes can be simply controlled by manipulating the precursor solution concentrations in a two-step sequential deposition process, thus achieving the feasible tunability of excitonic properties and lasing performance in hybrid metal-halide perovskites. The lasing threshold is at around 230 mu J cm(-2) in this solution-processed organic-inorganic lead-halide material, which is comparable to the colloidal quantum dot lasers. The efficient stimulated emission originates from the multiple random scattering provided by the micro-meter scale rugged morphology and polycrystalline grain boundaries. Thus the excitonic properties in perovskites exhibit high correlation with the formed morphology of the perovskite nanocrystals. Compared to the conventional lasers normally serving as a coherent light source, the perovskite random lasers are promising in making low-cost thin-film lasing devices for flexible and speckle-free imaging applications.
High-Operation-Temperature Plasmonic Nanolasers on Single-Crystalline Aluminum
(2016-05)
Chou, Yu-Hsun
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Wu, Yen-Mo
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Hong, Kuo-Bin
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Chou, Bo-Tsun
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Shih, Jheng-Hong
The recent development of plasmonics has overcome the optical diffraction limit and fostered the development of several important components including nanolasers, low-operation-power modulators, and high-speed detectors. In particular, the advent of surface-plasmon-polariton (SPP) nanolasers has enabled the development of coherent emitters approaching the nanoscale. SPP nanolasers widely adopted metal insulator semiconductor structures because the presence of an insulator can prevent large metal loss. However, the insulator is not necessary if permittivity combination of laser structures is properly designed. Here, we experimentally demonstrate a SPP nanolaser with a ZnO nanowire on the as-grown single-crystalline aluminum. The average lasing threshold of this simple structure is 20 MW/cm(2), which is four-times lower than that of structures with additional insulator layers. Furthermore, single-mode laser operation can be sustained at temperatures up to 353 K. Our study represents a major step toward the practical realization of SPP nanolasers.

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