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Single-crystalline aluminum film for ultraviolet plasmonic nanolasers
(2016-01-27)
Chou, Bo-Tsun
;
Chou, Yu-Hsun
;
Wu, Yen-Mo
;
Chung, Yi-Cheng
;
Hsueh, Wei-Jen
Significant advances have been made in the development of plasmonic devices in the past decade. Plasmonic nanolasers, which display interesting properties, have come to play an important role in biomedicine, chemical sensors, information technology, and optical integrated circuits. However, nanoscale plasmonic devices, particularly those operating in the ultraviolet regime, are extremely sensitive to the metal and interface quality. Thus, these factors have a significant bearing on the development of ultraviolet plasmonic devices. Here, by addressing these material-related issues, we demonstrate a low-threshold, high-characteristic-temperature metal-oxide-semiconductor ZnO nanolaser that operates at room temperature. The template for the ZnO nanowires consists of a flat single-crystalline Al film grown by molecular beam epitaxy and an ultrasmooth Al2O3 spacer layer synthesized by atomic layer deposition. By effectively reducing the surface plasmon scattering and metal intrinsic absorption losses, the high-quality metal film and the sharp interfaces formed between the layers boost the device performance. This work should pave the way for the use of ultraviolet plasmonic nanolasers and related devices in a wider range of applications.
Spin-orbit-coupled superconductivity
(2014-06-25)
Lo, Shun-Tsung
;
Lin, Shih-Wei
;
Wang, Yi-Ting
;
Lin, Sheng-Di
;
Liang, C. -T.
Superconductivity and spin-orbit (SO) interaction have been two separate emerging fields until very recently that the correlation between them seemed to be observed. However, previous experiments concerning SO coupling are performed far beyond the superconducting state and thus a direct demonstration of how SO coupling affects superconductivity remains elusive. Here we investigate the SO coupling in the critical region of superconducting transition on Al nanofilms, in which the strength of disorder and spin relaxation by SO coupling are changed by varying the film thickness. At temperatures T sufficiently above the superconducting critical temperature T-c, clear signature of SO coupling reveals itself in showing a magneto-resistivity peak. When T < T-c, the resistivity peak can still be observed; however, its line-shape is now affected by the onset of the quasi two-dimensional superconductivity. By studying such magneto-resistivity peaks under different strength of spin relaxation, we highlight the important effects of SO interaction on superconductivity.
Atomic-scale epitaxial aluminum film on GaAs substrate
(2017-07-01)
Fan, Yen-Ting
;
Lo, Ming-Cheng
;
Wu, Chu-Chun
;
Chen, Peng-Yu
;
Wu, Jenq-Shinn
Atomic-scale metal films exhibit intriguing size-dependent film stability, electrical conductivity, superconductivity, and chemical reactivity. With advancing methods for preparing ultra-thin and atomically smooth metal films, clear evidences of the quantum size effect have been experimentally collected in the past two decades. However, with the problems of small-area fabrication, film oxidation in air, and highly-sensitive interfaces between the metal, substrate, and capping layer, the uses of the quantized metallic films for further ex-situ investigations and applications have been seriously limited. To this end, we develop a large-area fabrication method for continuous atomic-scale aluminum film. The self-limited oxidation of aluminum protects and quantizes the metallic film and enables ex-situ characterizations and device processing in air. Structure analysis and electrical measurements on the prepared films imply the quantum size effect in the atomic-scale aluminum film. Our work opens the way for further physics studies and device applications using the quantized electronic states in metals. (C) 2017 Author(s).
Diamagnetic Response of Exciton Complexes in Semiconductor Quantum Dots
(2008-12-31)
Tsai, Ming-Fu
;
Lin, Hsuan
;
Lin, Chia-Hsien
;
Lin, Sheng-Di
;
Wang, Sheng-Yun
We report measurements of diamagnetic shifts for different exciton complexes confined in small InAs quantum dots. The measured diamagnetic responses are sensitive to the number of carriers in the exciton complexes, with systematic differences between neutral excitons, biexcitons, and trions. Theoretical calculations suggest that such systematic differences arise from very different extents of electron and hole wave functions confined in small quantum dots. The measured magnetic response of Coulomb energies is found to vary with the cube of the wave function extent, and can be a sensitive probe to the electron-hole wave function asymmetry.
Impacts of structural asymmetry on the magnetic response of excitons and biexcitons in single self-assembled In(Ga)As quantum rings
(2009-08-01)
Lin, Ta-Chun
;
Lin, Chia-Hsien
;
Ling, Hong-Shi
;
Fu, Ying-Jhe
;
Chang, Wen-Hao
The diamagnetic shifts of neutral excitons and biexcitons confined in single self-assembled In(Ga)As/GaAs quantum rings are investigated. Unlike quantum dots, quantum rings reveal a considerably large biexciton diamagnetic shift, about two times larger than that of single excitons. Based on model calculations, we found that the inherent structural asymmetry and imperfection, combined with the interparticle Coulomb interactions, is the fundamental cause of the more extended biexciton wave function in the quantum rings. The exciton wave function tends to be localized in one of the potential valleys induced by structural imperfections of the quantum ring due to the strong localization of hole and the electron-hole Coulomb attraction, resembling the behavior in single dots. Our results suggest that the phase coherence of neutral excitons in quantum rings will be smeared out by such wave function localizations.
Pure electron-electron dephasing in percolative aluminum ultrathin film grown by molecular beam epitaxy
(2015-02-18)
Lin, Shih-Wei
;
Wu, Yue-Han
;
Chang, Li
;
Liang, Chi-Te
;
Lin, Sheng-Di
We have successfully grown ultrathin continuous aluminum film by molecular beam epitaxy. This percolative aluminum film is single crystalline and strain free as characterized by transmission electron microscopy and atomic force microscopy. The weak anti-localization effect is observed in the temperature range of 1.4 to 10 K with this sample, and it reveals that, for the first time, the dephasing is purely caused by electron-electron inelastic scattering in aluminum.
Anticorrelation between the splitting and polarization of the exciton fine structure in single self-assembled InAs/GaAs quantum dots
(2011-02-28)
Lin, Chia-Hsien
;
You, Wen-Ting
;
Chou, Hsiang-Yu
;
Cheng, Shun-Jen
;
Lin, Sheng-Di
We report on a systematic correlation between the fine-structure splitting and polarization anisotropy of excitons in InAs/GaAs quantum dots, but with an unexpected reversal in order of the polarization eigenaxes. Such an anticorrelation is explained by a large valence-band-mixing induced splitting due to the shape and strain anisotropies. The strength and phase of valence band mixing are also found to play an important role in the tuning of fine structure splitting using an in-plane magnetic field.
Strong coupling of different cavity modes in photonic molecules formed by two adjacent microdisk microcavities
(2010-11-08)
Lin, Hsuan
;
Chen, Jhih-Hao
;
Chao, Shih-Shing
;
Lo, Ming-Cheng
;
Lin, Sheng-Di
Strong couplings between cavity modes in photonic molecules formed by two preselected nearly identical microdisk microcavities with embedded quantum dots are investigated. By continuously tuning the refractive index of one microdisk, clear anticrossings in the resonant peak energies associated with crossings in the peak linewidths can be observed. The coupling strengths are extracted by the coupled mode theory and analyzed by the model considering the effective potential confining the electromagnetic waves in the microcavities. (C) 2010 Optical Society of America
Ultrafast spin-polarized lasing in a highly photoexcited semiconductor microcavity at room temperature
(2015-05-14)
Hsu, Feng-kuo
;
Xie, Wei
;
Lee, Yi-Shan
;
Lin, Sheng-Di
;
Lai, Chih-Wei
We demonstrate room-temperature spin-polarized ultrafast (similar to 10 ps) lasing in a highly optically excited GaAs microcavity. This microcavity is embedded with InGaAs multiple quantum wells in which the spin relaxation time is less than 10 ps. The laser radiation remains highly circularly polarized even when excited by nonresonant elliptically polarized light. The lasing energy is not locked to the bare cavity resonance, and shifts similar to 10 meV as a function of the photoexcited density. Such spin-polarized lasing is attributed to a spin-dependent stimulated process of correlated electron-hole pairs. These pairs are formed near the Fermi edge in a high-density electron-hole plasma coupled to the cavity light field.
Surface roughness effects on aluminium-based ultraviolet plasmonic nanolasers
(2017-01-03)
Chung, Yi-Cheng
;
Cheng, Pi-Ju
;
Chou, Yu-Hsun
;
Chou, Bo-Tsun
;
Hong, Kuo-Bin
We systematically investigate the effects of surface roughness on the characteristics of ultraviolet zinc oxide plasmonic nanolasers fabricated on aluminium films with two different degrees of surface roughness. We demonstrate that the effective dielectric functions of aluminium interfaces with distinct roughness can be analysed from reflectivity measurements. By considering the scattering losses, including Rayleigh scattering, electron scattering, and grain boundary scattering, we adopt the modified Drude-Lorentz model to describe the scattering effect caused by surface roughness and obtain the effective dielectric functions of different Al samples. The sample with higher surface roughness induces more electron scattering and light scattering for SPP modes, leading to a higher threshold gain for the plasmonic nanolaser. By considering the pumping efficiency, our theoretical analysis shows that diminishing the detrimental optical losses caused by the roughness of the metallic interface could effectively lower (-33.1%) the pumping threshold of the plasmonic nanolasers, which is consistent with the experimental results.

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