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Optical, electro-optical, electrical and dielectric characterization of nematic liquid crystal (E7) layers doped with graphene nanoparticles for electro-optics
(2019-01-01)
Marinov, Y. G.
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Hadjichristov, G. B.
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Rafailov, P. M.
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Lin, S. H.
;
Marinova, V. M.
Thin (7 mu m) layers of nanocomposites from graphene nanoflakes (GrFs) dispersed at concentrations of 10(-3) wt.% into the nematic liquid crystal (NLC) E7 were characterized by various investigation techniques, such as Raman spectroscopy, impedance measurements and dielectric spectroscopy, as well as by electro-optical measurements (optical transmittance of the NLC layers versus the voltage of the applied external AC electric field). Conducting behaviour, dielectric permittivity and electric energy loss of our planar-aligned NLC layers at room temperature were analysed as a function of frequency in the range from 0.5 Hz to 1 MHz. The analysis of experimental data indicates that the molecular alignment through GrFs/NLC surface interactions is responsible for the reduction of the ionic conductivity of E7 NLC in the presence of GrFs. As compared to pure LC E7, this leads to improved characteristics for the studied nanocomposites, necessary in their practical applications in electro-optics.
Chemical vapour deposition growth and Raman characterization of graphene layers and carbon nanotubes
(2016-01-01)
Lai, Y-C
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Rafailov, P. M.
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Vlaikova, E.
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Marinova, V.
;
Lin, S. H.
Single-layer graphene films were grown by chemical vapour deposition (CVD) on Cu foil. The CVD process was complemented by plasma enhancement to grow also vertically aligned multiwalled carbon nanotubes using Ni nanoparticles as catalyst. The obtained samples were characterized by Raman spectroscopy analysis. Nature of defects in the samples and optimal growth conditions leading to achieve high quality of graphene and carbon nanotubes are discussed.
Liquid crystal cell with graphene electrodes
(2017-01-01)
Marinova, V.
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Tong, Z. F.
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Petrov, S.
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Lin, S. H.
;
Chen, M. S.
We demonstrate a graphene-based nematic liquid crystal cells fabricated by photo alignment technique. The modulation characteristics have been measured revealing that photo alignment method shows great potential for protecting the graphene layer on glass substrate during LC device fabrication.
Adiabatic treatment for vibrational predissociation of water dimers with channel interactions
(2015-01-01)
Mineo, H.
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Lin, S. H.
;
Fujimura, Y.
;
應用化學系
;
應用化學系分子科學碩博班
The results of calculated vibrational predissociation (VPD) of water dimers are presented. The VPD processes considered here are the followings: initially closed channel of symmetric stretching mode is excited by one quantum, and dissociate to two open channels of the bending mode excitation by one quantum in the donor and acceptor units. The VPD rate constants are calculated in the quantum mechanical approach under the adiabatic approximation. The channel interactions were taken into account in and between the initial and final states. The results obtained by quantum-mechanical approach are compared with both experimental and semi-classical trajectory calculation results.
Influence of neighboring levels in three-pulse photon-echo processes
(2009-05-01)
Villaeys, A. A.
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Dappe, Y. J.
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Liang, K. K.
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Lin, S. H.
;
應用化學系
It is the purpose of the present paper to study the dynamics underlying a three-pulse photon-echo process performed on a vibronic system coupled to non-Markovian baths, when a neighboring level enters into the global dynamical evolution because of broadband excitation required in these experiments. Particular emphasis is on the energy gap between the vibronic levels, but also on the fluctuation amplitudes and correlation times of their corresponding thermal baths. The photon-echo signal appears to be very sensitive to the additional interfering contributions introduced by the neighboring vibronic level. It is shown that these contributions associated to the pathways involving different vibronic states are modulated by their corresponding energy gap. As a consequence, these contributions to the integrated photon-echo signal strongly decrease for large energy gaps. Also, an oscillating behavior is observed on the time dependence of the photon-echo signal resulting from the summation of the contributions provided by the individual vibronic levels. Moreover, the influence of the non-Markovian character of the baths, accountable for inhomogeneous broadening, affects the amplitude and the time dependence of the photon-echo signal, as well as its dependence with the delay time of the laser pulses. Of course, for longer times a Markovian dynamical evolution is recovered.
Adiabatically slow and adiabatically fast driven ratchets
(2012-04-12)
Rozenbaum, V. M.
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Makhnovskii, Yu. A.
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Shapochkina, I. V.
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Sheu, S. -Y.
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Yang, D. -Y.
We revisit two known models of deterministically driven ratchets, which exhibit high energetic efficiency, with the goal to uncover similarities and differences in the principles of their operation. Both the models rely on adiabaticity of the potential change process, however, the adiabaticity that we deal with in the two cases is of different types, slow and fast. It is shown that in the former (latter) case the drift velocity is an even (odd) functional of the potential, with the notable consequence that for the adiabatically slow driven ratchet the necessary symmetry breaking occurs only due to time-dependent parametric perturbations, while the spatial asymmetry of the potential is a mandatory condition for the adiabatically fast driven ratchet to operate. To treat energetic characteristics, the models are restated in terms of traveling potential ratchets. With such an approach, we find that in these cases (i) the conditions of high energetic efficiency to be reached are similar, and (ii) the symmetry properties of the kinetic coefficients are different. Based on our results, a strategy for designing efficient Brownian motors is suggested.
Two-state Brownian motor driven by synchronously fluctuating unbiased forces
(2011-08-04)
Rozenbaum, V. M.
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Makhnovskii, Yu A.
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Sheu, S. -Y.
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Yang, D. -Y.
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Lin, S. H.
As a model of the Brownian motor, we consider a particle moving unidirectionally under the action of two synchronously fluctuating unbiased forces, transverse and longitudinal with respect to the particle track. The former force induces track-normal transitions of the particle between the attached and detached states (with and without a periodic potential, respectively), whereas the latter drives track-parallel motion in either state. Analytical expressions of the current and efficiency are derived for different regimes, with due account of the delayed response of the system to force fluctuations. For a sawtooth potential in the attached state, we reveal several motion regimes affording the maximum current or the maximum efficiency. A special emphasis is placed on the possibility of current reversal. As shown, the interplay between two phase-shifted harmonically varied forces as well as inherent and externally induced asymmetry can lead to the emergence of multiple current reversals, thus enabling the flexible controllability of the motion direction.
The influence of Rh doping on the light-induced properties of Bi4Ge3O12 single crystals
(2009-01-01)
Marinova, V.
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Petrova, D.
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Lin, S. H.
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Hsieh, M. L.
;
Hsu, K. Y.
The influence of different doping concentrations of rhodium on the light-induced and holographic properties of BGO crystal is investigated. It is found that Rh addition generates sufficient density of traps for photoinduced charge carriers such that holographic gratings are successfully recorded in the blue-green spectral range. The measured steady state diffraction efficiency at 514 nm is 0.14%, which corresponds to a refractive index modulation of Delta n similar to 1.5 x 10(-6) for higher Rh concentration. A photochromic effect and nonlinear dependence of photoconductivity on light intensity are observed indicating deep level and shallow level contributions to the charge transport mechanism of Rh-doped BGO.
Low-V-t TaN/HfLaO n-MOSFETs Using Low-Temperature Formed Source-Drain Junctions
(2009-01-01)
Lin, S. H.
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Liu, S. L.
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Yeh, F. S.
;
Chin, Albert
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電子工程學系及電子研究所
We report low-threshold-voltage (V-t) TaN/HfLaO n-MOSFETs using solid-phase-diffusion (SPD)-formed junctions at a low temperature of 650 degrees C. The gate-first and self-aligned TaN/HflLaO n-MOSFETs using Ni/Sb SPID-formed source-drain junctions showed a low Vt of 0.16 V and a peak electron mobility of 187 cm(2)/V . s at a small 1.3-nm equivalent oxide thickness.
Structure and predissociation of the 3p sigma(u)D (3)Sigma(+)(u) Rydberg state of N(2): First extreme-ultraviolet and new near-infrared observations, with coupled-channels analysis
(2008-11-28)
Wang, Qiaoqiao
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Wu, Di
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Jin, Mingxing
;
Liu, Fuchun
;
Hu, Feifei
The 3p sigma(u)D (3)Sigma(+)(u) Rydberg state of N(2) is studied experimentally using two high-resolution spectroscopic techniques. First, the forbidden D (3)Sigma(+)(u)-X (1)Sigma(+)(g) transition is observed for the first time via the (0,0) band of (14)N(2) and the (1,0) band of (15)N(2), using 1 extreme-ultraviolet +1 ultraviolet two-photon-ionization laser spectroscopy. Second, the Rydberg-Rydberg transition D (3)Sigma(+)(u)-E (3)Sigma(+)(g) is studied using near-infrared diode-laser photoabsorption spectroscopy, thus extending the previous measurements of Kanamori [J. Chem. Phys. 95, 80 (1991)], to higher transition energies, and thereby revealing the (2,2) and (3,3) bands. The combined results show that the D(v=0-3) levels exhibit rapidly increasing rotational predissociation as v increases, spanning nearly four orders of magnitude. The D-state level structure and rotational predissociation signature are explained by means of a coupled-channels model which considers the electrostatically coupled (3)Pi(u) Rydberg-valence manifold, together with a pure-precession L-uncoupling rotational interaction between the 3p sigma(u)D (3)Sigma(+)(u) and 3p pi(u)G (3)Pi(u) Rydberg p-complex components.

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