標題: Diffusion of a massive particle in a periodic potential: Application to adiabatic ratchets
作者: Rozenbaum, Viktor M.
Makhnovskii, Yurii A.
Shapochkina, Irina V.
Sheu, Sheh-Yi
Yang, Dah-Yen
Lin, Sheng Hsien
應用化學系
Department of Applied Chemistry
公開日期: 18-十二月-2015
摘要: We generalize a theory of diffusion of a massive particle by the way in which transport characteristics are described by analytical expressions that formally coincide with those for the overdamped massless case but contain a factor comprising the particle mass which can be calculated in terms of Risken's matrix continued fraction method (MCFM). Using this generalization, we aim to elucidate how large gradients of a periodic potential affect the current in a tilted periodic potential and the average current of adiabatically driven on-off flashing ratchets. For this reason, we perform calculations for a sawtooth potential of the period L with an arbitrary sawtooth length (l < L) instead of the smooth potentials typically considered in MCFM-solvable problems. We find nonanalytic behavior of the transport characteristics calculated for the sharp extremely asymmetric sawtooth potential at l -> 0 which appears due to the inertial effect. Analysis of the temperature dependences of the quantities under study reveals the dominant role of inertia in the high-temperature region. In particular, we show, by the analytical strong-inertia approach developed for this region, that the temperature-dependent contribution to the mobility at zero force and to the related effective diffusion coefficient are proportional to T-3/2 and T-1/2, respectively, and have a logarithmic singularity at l -> 0.
URI: http://dx.doi.org/10.1103/PhysRevE.92.062132
http://hdl.handle.net/11536/129530
ISSN: 1539-3755
DOI: 10.1103/PhysRevE.92.062132
期刊: PHYSICAL REVIEW E
Volume: 92
Issue: 6
起始頁: 0
結束頁: 0
顯示於類別:期刊論文


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