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dc.contributor.authorYamaki, Masahiroen_US
dc.contributor.authorMineo, Hirobumien_US
dc.contributor.authorTeranishi, Yoshiakien_US
dc.contributor.authorLin, Sheng Hsienen_US
dc.contributor.authorFujimura, Yuichien_US
dc.date.accessioned2016-03-28T00:04:27Z-
dc.date.available2016-03-28T00:04:27Z-
dc.date.issued2016-01-01en_US
dc.identifier.issn0009-4536en_US
dc.identifier.urihttp://dx.doi.org/10.1002/jccs.201500043en_US
dc.identifier.urihttp://hdl.handle.net/11536/129697-
dc.description.abstractControl of mobile -electrons is one of the fundamental issues in the organic optoelectronics for designing the next generation ultrafast switching devices. The optimal control simulations of coherent -electron rotations in (P)-2,2\'-biphenol, which is the typical nonplanar aromatic molecule with axial chirality, were performed by taking into account two types of the control targets: one is generation of the maximum -angular momentum, and the other is the maintaining of the generated unidirectional angular momentum during a setting time duration. The optimal control pulse for each target is designed. The analysis of the simulation results shows that the effective maintaining of the unidirectional angular momentum can be realized by applying 2 pulse to one of the electronic excited states forming the coherent electronic state. The 2 pulse prevents the reverse rotation of the -electrons by dumping the excited state population to the ground state and subsequently by pumping the population back to the excited state. The present results provide a theoretical basis for the designing next generation ultrafast switching devices made by organic aromatic molecules.en_US
dc.language.isoen_USen_US
dc.subjectQuantum controlen_US
dc.subject(P)-2en_US
dc.subject2'-biphenolen_US
dc.subject-electronen_US
dc.subjectAngular momentumen_US
dc.subjectRing currenten_US
dc.subject2 pulseen_US
dc.titleQuantum Control of Coherent -Electron Dynamics in Chiral Aromatic Moleculesen_US
dc.typeArticleen_US
dc.identifier.doi10.1002/jccs.201500043en_US
dc.identifier.journalJOURNAL OF THE CHINESE CHEMICAL SOCIETYen_US
dc.citation.volume63en_US
dc.citation.spage87en_US
dc.citation.epage92en_US
dc.contributor.department應用化學系分子科學碩博班zh_TW
dc.contributor.department物理研究所zh_TW
dc.contributor.departmentInstitute of Molecular scienceen_US
dc.contributor.departmentInstitute of Physicsen_US
dc.identifier.wosnumberWOS:000369014800008en_US
dc.citation.woscount0en_US
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