Full metadata record
DC FieldValueLanguage
dc.contributor.authorShown, Indrajiten_US
dc.contributor.authorSamireddi, Satyanarayanaen_US
dc.contributor.authorChang, Yu-Chungen_US
dc.contributor.authorPutikam, Raghunathen_US
dc.contributor.authorChang, Po-Hanen_US
dc.contributor.authorSabbah, Amren_US
dc.contributor.authorFu, Fang-Yuen_US
dc.contributor.authorChen, Wei-Fuen_US
dc.contributor.authorWu, Chih-Ien_US
dc.contributor.authorYu, Tsyr-Yanen_US
dc.contributor.authorChung, Po-Wenen_US
dc.contributor.authorLin, M. C.en_US
dc.contributor.authorChen, Li-Chyongen_US
dc.contributor.authorChen, Kuei-Hsienen_US
dc.date.accessioned2018-08-21T05:53:11Z-
dc.date.available2018-08-21T05:53:11Z-
dc.date.issued2018-01-12en_US
dc.identifier.issn2041-1723en_US
dc.identifier.urihttp://dx.doi.org/10.1038/s41467-017-02547-4en_US
dc.identifier.urihttp://hdl.handle.net/11536/144366-
dc.description.abstractPhotocatalytic formation of hydrocarbons using solar energy via artificial photosynthesis is a highly desirable renewable-energy source for replacing conventional fossil fuels. Using an L-cysteine-based hydrothermal process, here we synthesize a carbon-doped SnS2 (SnS2-C) metal dichalcogenide nanostructure, which exhibits a highly active and selective photocatalytic conversion of CO2 to hydrocarbons under visible-light. The interstitial carbon doping induced microstrain in the SnS2 lattice, resulting in different photophysical properties as compared with undoped SnS2. This SnS2-C photocatalyst significantly enhances the CO2 reduction activity under visible light, attaining a photochemical quantum efficiency of above 0.7%. The SnS2-C photocatalyst represents an important contribution towards high quantum efficiency artificial photosynthesis based on gas phase photocatalytic CO2 reduction under visible light, where the in situ carbon-doped SnS2 nanostructure improves the stability and the light harvesting and charge separation efficiency, and significantly enhances the photocatalytic activity.en_US
dc.language.isoen_USen_US
dc.titleCarbon-doped SnS2 nanostructure as a high-efficiency solar fuel catalyst under visible lighten_US
dc.typeArticleen_US
dc.identifier.doi10.1038/s41467-017-02547-4en_US
dc.identifier.journalNATURE COMMUNICATIONSen_US
dc.citation.volume9en_US
dc.contributor.department應用化學系zh_TW
dc.contributor.departmentDepartment of Applied Chemistryen_US
dc.identifier.wosnumberWOS:000419949100003en_US
Appears in Collections:Articles