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dc.contributor.authorMakhnovskii, Yurii A.en_US
dc.contributor.authorSheu, Sheh-Yien_US
dc.contributor.authorYang, Dah-Yenen_US
dc.contributor.authorLin, Sheng Hsienen_US
dc.date.accessioned2018-08-21T05:53:58Z-
dc.date.available2018-08-21T05:53:58Z-
dc.date.issued2017-04-21en_US
dc.identifier.issn0021-9606en_US
dc.identifier.urihttp://dx.doi.org/10.1063/1.4979984en_US
dc.identifier.urihttp://hdl.handle.net/11536/145416-
dc.description.abstractThe motion of a spherical Brownian particle in an asymmetric periodic channel is considered. Under an external periodic stimulus, the particle switches between two states with different particle radius, every half-period. Using Brownian dynamics simulations, we show that the particle size oscillation, combined with the asymmetry of the channel, induces a drift along the channel axis, directed towards the steeper wall of the channel. The oscillation of the particle size is accompanied by a time variation of the space accessible to the particle and by an oscillation of its diffusion coefficient. The former underlies the drift inducing mechanism of purely entropic nature. The latter, combined with the former, leads to a significant amplification of the effect. The drift velocity vanishes when interconversion between the states occurs either very slow or very fast, having a maximum in between. The position and magnitude of the maximum are discussed by providing an analytical approach based on intuitively appealing assumptions. Published by AIP Publishing.en_US
dc.language.isoen_USen_US
dc.titleDirected motion from particle size oscillations inside an asymmetric channelen_US
dc.typeArticleen_US
dc.identifier.doi10.1063/1.4979984en_US
dc.identifier.journalJOURNAL OF CHEMICAL PHYSICSen_US
dc.citation.volume146en_US
dc.contributor.department應用化學系zh_TW
dc.contributor.departmentDepartment of Applied Chemistryen_US
dc.identifier.wosnumberWOS:000399904500004en_US
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