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dc.contributor.authorYamaki, Masahiroen_US
dc.contributor.authorMineo, Hirobumien_US
dc.contributor.authorTeranishi, Yoshiakien_US
dc.contributor.authorHayashi, Michitoshien_US
dc.contributor.authorFujimura, Yuichien_US
dc.contributor.authorNakamura, Hirokien_US
dc.contributor.authorLin, Sheng Hsienen_US
dc.date.accessioned2019-04-02T06:01:03Z-
dc.date.available2019-04-02T06:01:03Z-
dc.date.issued2014-06-05en_US
dc.identifier.issn1948-7185en_US
dc.identifier.urihttp://dx.doi.org/10.1021/jz5007109en_US
dc.identifier.urihttp://hdl.handle.net/11536/147690-
dc.description.abstractControlling g-electrons with delocalized character is one of the fundamental issues in femtosecond and attosecond chemistry. Localization of pi-electron rotation by using laser pulses is expected to play an essential role in nanoscience. The pi-electron rotation created at a selected aromatic ring of a single molecule induces a local intense electromagnetic field, which is a new type of ultrafast optical control functioning. We propose a quantum localization of coherent pi-electron angular momentum in (P)-2,2'-biphenol, which is a simple, covalently linked chiral aromatic ring chain molecule. The localization considered here consists of sequential two steps: the first step is to localize the pi-electron angular momentum at a selected ring of the two benzene rings, and the other is to maintain the localization. Optimal control theory was used for obtaining the optimized electric fields of linearly polarized laser pulses to realize the localization. The optimal electric fields and the resultant coherent electronic dynamics are analyzed.en_US
dc.language.isoen_USen_US
dc.titleQuantum Localization of Coherent pi-Electron Angular Momentum in (P)-2,2 '-Biphenolen_US
dc.typeArticleen_US
dc.identifier.doi10.1021/jz5007109en_US
dc.identifier.journalJOURNAL OF PHYSICAL CHEMISTRY LETTERSen_US
dc.citation.volume5en_US
dc.citation.spage2044en_US
dc.citation.epage2049en_US
dc.contributor.department應用化學系分子科學碩博班zh_TW
dc.contributor.department物理研究所zh_TW
dc.contributor.departmentInstitute of Molecular scienceen_US
dc.contributor.departmentInstitute of Physicsen_US
dc.identifier.wosnumberWOS:000337012500043en_US
dc.citation.woscount13en_US
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