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dc.contributor.authorKobayashi, Takayoshien_US
dc.contributor.authorYamashita, Munenorien_US
dc.contributor.authorDu, Juanen_US
dc.contributor.authorZhang, Junen_US
dc.contributor.authorIwakura, Izumien_US
dc.date.accessioned2014-12-08T15:31:08Z-
dc.date.available2014-12-08T15:31:08Z-
dc.date.issued2013-07-30en_US
dc.identifier.issn0009-2614en_US
dc.identifier.urihttp://dx.doi.org/10.1016/j.cplett.2013.06.029en_US
dc.identifier.urihttp://hdl.handle.net/11536/22178-
dc.description.abstractThe electronic population decay time is determined to be about 500 fs in (poly-[2-methoxy-5-(2'-ethyl-hexyloxy)-p-phenylenevinylenel (MEH-PPV) using 5.7 fs pulses. The ultrafast electronic dephasing time and the self-trapping time of free exciton to form an exciton polaron is determined as 25 +/- 2 fs and 50 +/- 23 fs, respectively. Real-time spectrogram analysis reveals dynamic mode coupling among the high-frequency and low-frequency modes. The energy-ladder descent vibrational process is clarified using the first moment of the difference absorption spectrum. The phase relaxation time is calculated from the widths of the Fourier spectra of several strongly coupled modes. (C) 2013 Elsevier B.V. All rights reserved.en_US
dc.language.isoen_USen_US
dc.titleVibrational and electronic relaxation in MEH-PPV using few cycle pulsesen_US
dc.typeArticleen_US
dc.identifier.doi10.1016/j.cplett.2013.06.029en_US
dc.identifier.journalCHEMICAL PHYSICS LETTERSen_US
dc.citation.volume579en_US
dc.citation.issueen_US
dc.citation.spage51en_US
dc.citation.epage57en_US
dc.contributor.department電子物理學系zh_TW
dc.contributor.departmentDepartment of Electrophysicsen_US
dc.identifier.wosnumberWOS:000322558200009-
dc.citation.woscount0-
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