完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.author | Yamaki, Masahiro | en_US |
dc.contributor.author | Mineo, Hirobumi | en_US |
dc.contributor.author | Teranishi, Yoshiaki | en_US |
dc.contributor.author | Hayashi, Michitoshi | en_US |
dc.contributor.author | Fujimura, Yuichi | en_US |
dc.contributor.author | Nakamura, Hiroki | en_US |
dc.contributor.author | Lin, Sheng Hsien | en_US |
dc.date.accessioned | 2014-12-08T15:36:19Z | - |
dc.date.available | 2014-12-08T15:36:19Z | - |
dc.date.issued | 2014-06-05 | en_US |
dc.identifier.issn | 1948-7185 | en_US |
dc.identifier.uri | http://dx.doi.org/10.1021/jz5007109 | en_US |
dc.identifier.uri | http://hdl.handle.net/11536/24649 | - |
dc.description.abstract | Controlling g-electrons with delocalized character is one of the fundamental issues in femtosecond and attosecond chemistry. Localization of pi-electron rotation by using laser pulses is expected to play an essential role in nanoscience. The pi-electron rotation created at a selected aromatic ring of a single molecule induces a local intense electromagnetic field, which is a new type of ultrafast optical control functioning. We propose a quantum localization of coherent pi-electron angular momentum in (P)-2,2\'-biphenol, which is a simple, covalently linked chiral aromatic ring chain molecule. The localization considered here consists of sequential two steps: the first step is to localize the pi-electron angular momentum at a selected ring of the two benzene rings, and the other is to maintain the localization. Optimal control theory was used for obtaining the optimized electric fields of linearly polarized laser pulses to realize the localization. The optimal electric fields and the resultant coherent electronic dynamics are analyzed. | en_US |
dc.language.iso | en_US | en_US |
dc.title | Quantum Localization of Coherent pi-Electron Angular Momentum in (P)-2,2 \'-Biphenol | en_US |
dc.type | Article | en_US |
dc.identifier.doi | 10.1021/jz5007109 | en_US |
dc.identifier.journal | JOURNAL OF PHYSICAL CHEMISTRY LETTERS | en_US |
dc.citation.volume | 5 | en_US |
dc.citation.issue | 11 | en_US |
dc.citation.spage | 2044 | en_US |
dc.citation.epage | 2049 | en_US |
dc.contributor.department | 應用化學系分子科學碩博班 | zh_TW |
dc.contributor.department | 物理研究所 | zh_TW |
dc.contributor.department | Institute of Molecular science | en_US |
dc.contributor.department | Institute of Physics | en_US |
顯示於類別: | 期刊論文 |