標題: | Photoinduced multimode coherent acoustic phonons of metallic nanoprisms and the effects of shape-induced anisotropic electronic stresses |
作者: | Tai, Po-Tse Yu, Pyng Tang, Jau 光電工程學系 Department of Photonics |
公開日期: | 14-五月-2011 |
摘要: | In this work we reported experimental measurements of ultrafast structural dynamics in metallic nanoprisms induced by a femtosecond laser pulse. The main focus of this study of anisotropic heating in nanoprisms is about laser fluence effects on photoexcitation of two planar coherent acoustic phonon modes, namely, the breathing mode and the totally symmetric mode. We presented a combined two-temperature model and 2-D Fermi-Pasta-Ulam model to explain both the dependence of the initial phases and the mode weight on the excitation power. Our transient optical absorption data for both the initial fast monotonic decay and the subsequent coherent acoustic oscillations clearly indicate the presence of anisotropic thermal expansion in nanoprisms. (C) 2011 American Institute of Physics. [doi:10.1063/1.3590373] |
URI: | http://dx.doi.org/10.1063/1.3590373 http://hdl.handle.net/11536/8861 |
ISSN: | 0021-9606 |
DOI: | 10.1063/1.3590373 |
期刊: | JOURNAL OF CHEMICAL PHYSICS |
Volume: | 134 |
Issue: | 18 |
結束頁: | |
顯示於類別: | 期刊論文 |