Excited-state molecular vibration observed for a probe pulse preceding the pump pulse by real-time optical spectroscopy
| dc.citation.epage | 0 | en_US |
| dc.citation.issue | 3 | en_US |
| dc.citation.spage | 0 | en_US |
| dc.citation.volume | 101 | en_US |
| dc.citation.woscount | 25 | en_US |
| dc.contributor.author | Kobayashi, Takayoshi | en_US |
| dc.contributor.author | Du, Juan | en_US |
| dc.contributor.author | Feng, Wei | en_US |
| dc.contributor.author | Yoshino, Katsumi | en_US |
| dc.contributor.department | 電子物理學系 | zh_TW |
| dc.contributor.department | Department of Electrophysics | en_US |
| dc.date.accessioned | 2019-04-03T06:40:28Z | |
| dc.date.available | 2019-04-03T06:40:28Z | |
| dc.date.issued | 2008-07-18 | en_US |
| dc.description.abstract | It is shown experimentally that the absorbance change observed in the "negative" time range, where probe pulse precedes pump pulse in real-time vibrational spectroscopy is induced only by the excited-state wave-packet motion as theoretically expected. Coherent molecular vibration of a polymer in the excited state was observed in the real-time trace without the effect of wave-packet motion in the ground state, which usually makes it difficult to ascribe the signal either to the ground state or to the excited state. | en_US |
| dc.identifier.doi | 10.1103/PhysRevLett.101.037402 | en_US |
| dc.identifier.issn | 0031-9007 | en_US |
| dc.identifier.journal | PHYSICAL REVIEW LETTERS | en_US |
| dc.identifier.uri | http://dx.doi.org/10.1103/PhysRevLett.101.037402 | en_US |
| dc.identifier.uri | https://ir.lib.nycu.edu.tw/handle/11536/8564 | |
| dc.identifier.wosnumber | WOS:000258184500057 | en_US |
| dc.language.iso | en_US | en_US |
| dc.title | Excited-state molecular vibration observed for a probe pulse preceding the pump pulse by real-time optical spectroscopy | en_US |
| dc.type | Article | en_US |