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Study of fluorescence enhancement of colloidal CdSe/ZnS quantum dots bound to hexadecylamine by single-molecule measurements

dc.citation.epage15172en_US
dc.citation.issue42en_US
dc.citation.spage15166en_US
dc.citation.volume111en_US
dc.citation.woscount16
dc.contributor.authorYuan, Chi-Tsuen_US
dc.contributor.authorChou, Wu-Chingen_US
dc.contributor.authorChen, Yueh-Nanen_US
dc.contributor.authorChou, Jui-Wenen_US
dc.contributor.authorChuuji, Der-Sanen_US
dc.contributor.authorLin, Cheng-An J.en_US
dc.contributor.authorLi, Jimmy K.en_US
dc.contributor.authorChang, Walter H.en_US
dc.contributor.authorShen, Ji-Linen_US
dc.contributor.department電子物理學系zh_TW
dc.contributor.departmentDepartment of Electrophysicsen_US
dc.date.accessioned2014-12-08T15:13:14Z
dc.date.available2014-12-08T15:13:14Z
dc.date.issued2007-10-25en_US
dc.description.abstractFluorescence enhancement of colloidal CdSe/ZnS quantum dots (QDs) by the binding of hexadecylamine (HDA) ligands was investigated at the single-QD level. The blinking behavior of individual CdSe/ZnS QDs can be dramatically modified by additional HDA ligands. Both the ratio of the mean on/off time lengths and the total number of emitted photons within the on-time duration can be enhanced, by factors of up to 2.8 and 13, respectively. Consequently, the blinking rate can be suppressed down to 18%. The fluorescence decay curve is closer to a single-exponential decay profile and has a longer measured lifetime. These results suggest that HDA ligands can further improve surface passivation.en_US
dc.identifier.doi10.1021/jp074561pen_US
dc.identifier.issn1932-7447en_US
dc.identifier.journalJOURNAL OF PHYSICAL CHEMISTRY Cen_US
dc.identifier.urihttp://dx.doi.org/10.1021/jp074561pen_US
dc.identifier.urihttps://ir.lib.nycu.edu.tw/handle/11536/10221
dc.identifier.wosnumberWOS:000250438900007
dc.language.isoen_USen_US
dc.titleStudy of fluorescence enhancement of colloidal CdSe/ZnS quantum dots bound to hexadecylamine by single-molecule measurementsen_US
dc.typeArticleen_US

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