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THEORY OF DOUBLY RESONANT INFRARED-VISIBLE SUM-FREQUENCY AND DIFFERENCE-FREQUENCY-GENERATION FROM ADSORBED MOLECULES

dc.citation.epage3981en_US
dc.citation.issue5en_US
dc.citation.spage3973en_US
dc.citation.volume49en_US
dc.citation.woscount47en_US
dc.contributor.authorHUANG, JYen_US
dc.contributor.authorSHEN, YRen_US
dc.contributor.department光電工程研究所zh_TW
dc.contributor.departmentInstitute of EO Enginerringen_US
dc.date.accessioned2019-04-03T06:39:09Z
dc.date.available2019-04-03T06:39:09Z
dc.date.issued1994-05-01en_US
dc.description.abstractWe theoretically analyze doubly resonant infrared-visible sum-frequency (DR IVSFG) and difference-frequency generation (DR IVDFG) from a monolayer of adsorbates at an interface. our calculated results with a model molecule indicate that the resonant amplitude of nonlinear optical susceptibility of DR IVDFG and DR IVSFG processes conveys information about the electron-vibration coupling in adsorbates. Moreover, owing to a dephasing-rephasing procedure involved, DR IVDFG can also be developed into a sensitive probe for investigating the coherent phase relaxation process in adsorbed molecules without the complication of inhomogeneous broadening.en_US
dc.identifier.doi10.1103/PhysRevA.49.3973en_US
dc.identifier.issn1050-2947en_US
dc.identifier.journalPHYSICAL REVIEW Aen_US
dc.identifier.urihttp://dx.doi.org/10.1103/PhysRevA.49.3973en_US
dc.identifier.urihttps://ir.lib.nycu.edu.tw/handle/11536/2499
dc.identifier.wosnumberWOS:A1994NL38600019en_US
dc.language.isoen_USen_US
dc.titleTHEORY OF DOUBLY RESONANT INFRARED-VISIBLE SUM-FREQUENCY AND DIFFERENCE-FREQUENCY-GENERATION FROM ADSORBED MOLECULESen_US
dc.typeArticleen_US

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