Experimental and theoretical investigation of high-power laser ionization and dissociation of methane
| dc.citation.epage | 9416 | en_US |
| dc.citation.issue | 38 | en_US |
| dc.citation.spage | 9405 | en_US |
| dc.citation.volume | 111 | en_US |
| dc.citation.woscount | 8 | |
| dc.contributor.author | Sharifi, A. | en_US |
| dc.contributor.author | Kong, F. | en_US |
| dc.contributor.author | Chin, S. L. | en_US |
| dc.contributor.author | Mineo, H. | en_US |
| dc.contributor.author | Dyakov, Y. | en_US |
| dc.contributor.author | Mebel, A. M. | en_US |
| dc.contributor.author | Chao, S. D. | en_US |
| dc.contributor.author | Hayashi, M. | en_US |
| dc.contributor.author | Lin, S. H. | en_US |
| dc.contributor.department | 應用化學系 | zh_TW |
| dc.contributor.department | Department of Applied Chemistry | en_US |
| dc.date.accessioned | 2014-12-08T15:13:20Z | |
| dc.date.available | 2014-12-08T15:13:20Z | |
| dc.date.issued | 2007-09-27 | en_US |
| dc.description.abstract | The main purpose of this paper is to report the high-power laser ionization-dissociation of CH4 at various femtosecond (fs) laser intensities (from 1 x 10 14 W/cm(2) to 2 x 1015 W/cm(2)) with a laser pulse duration of 48 fs. The generalized molecular Keldysh theory has been applied to calculate the ionization yields for CH4+ and CH4++. Outside the influence of the A intense laser, we propose to calculate the mass spectra due to the decomposition of CH4+ and CH4++, using the Rice-Ramsperger-Kassel-Marcus (RRKM) theory. The agreement between the experimental mass spectra and calculated mass spectra seems to be reasonable. | en_US |
| dc.identifier.doi | 10.1021/jp074053f | en_US |
| dc.identifier.issn | 1089-5639 | en_US |
| dc.identifier.journal | JOURNAL OF PHYSICAL CHEMISTRY A | en_US |
| dc.identifier.uri | http://dx.doi.org/10.1021/jp074053f | en_US |
| dc.identifier.uri | https://ir.lib.nycu.edu.tw/handle/11536/10308 | |
| dc.identifier.wosnumber | WOS:000249655600031 | |
| dc.language.iso | en_US | en_US |
| dc.title | Experimental and theoretical investigation of high-power laser ionization and dissociation of methane | en_US |
| dc.type | Article | en_US |