標題: Theory of time-resolved sum-frequency generation and its applications to vibrational dynamics of water
作者: Hayashi, Michitoshi
Shiu, Ying-Jen
Liang, Kuo Kan
Lin, Sheng Hsien
Shen, Yuan Ron
應用化學系
Department of Applied Chemistry
公開日期: 20-Sep-2007
摘要: A molecular theory of time-resolved sum-frequency generation (SFG) has been developed. The theoretical framework is constructed using the coupled-oscillator model in the adiabatic approximation. This theory can treat not only the vibrational spectroscopy but also vibrational dynamics. An application of this theory is also provided for estimation of the time constants of the intermolecular vibrational energy transfer between water molecules. This approach can be used for molecular analysis of the experimental results of Shen at al. on the SFG studies of vibrational dynamics of water.
URI: http://dx.doi.org/10.1021/jp0708300
http://hdl.handle.net/11536/10324
ISSN: 1089-5639
DOI: 10.1021/jp0708300
期刊: JOURNAL OF PHYSICAL CHEMISTRY A
Volume: 111
Issue: 37
起始頁: 9062
結束頁: 9069
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