完整後設資料紀錄
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dc.contributor.authorDhole, Sandipen_US
dc.contributor.authorSelvaraju, Manikandanen_US
dc.contributor.authorMaiti, Barnalien_US
dc.contributor.authorChanda, Kaushiken_US
dc.contributor.authorSun, Chung-Mingen_US
dc.date.accessioned2015-07-21T08:29:39Z-
dc.date.available2015-07-21T08:29:39Z-
dc.date.issued2015-05-01en_US
dc.identifier.issn2156-8952en_US
dc.identifier.urihttp://dx.doi.org/10.1021/acscombsci.5b00010en_US
dc.identifier.urihttp://hdl.handle.net/11536/124835-
dc.description.abstractAn efficient cascade synthesis of novel benzimidazole linked alkyloxypyrrolo[1,2-a]quinoxalinones was explored on soluble polymer support under micro-Wave irradiation. Two exclusive protocols have been developed for the partial and reductive cyclization by Controlling the microwave energy, Commencing from the smile substrate, ortho nitro, pyrrol: carboxylates, N-hydroxy pyrroloquinoxalinones were obtained by,, partial reductive cyclization (60 degrees C, 7 min), and the synthesis of pyrroloquinoxalinones was accomplished by full reductive, cyclization (85 degrees C, 12 min). This method represents the first synthesis N-hydroxy pyrroloquinoxalinones using Pd/C and ammonium formate as reducing agents: Further employing a variety Of alkyl bromides, the obtained pyrroloquinoxalinones were transformed to their corresponding O-, and N-alkylated analogues to deliver the diversified, novel molecular entities.en_US
dc.language.isoen_USen_US
dc.subjectpolymer supporteden_US
dc.subjectmicrowave-assisteden_US
dc.subjectpyrroloquinoxalinonesen_US
dc.subjectreductive cyclizationen_US
dc.titleMicrowave Controlled Reductive Cyclization: A Selective Synthesis of Novel Benzimidazole-alkyloxypyrrolo[1,2-a]quinoxalinonesen_US
dc.typeArticleen_US
dc.identifier.doi10.1021/acscombsci.5b00010en_US
dc.identifier.journalACS COMBINATORIAL SCIENCEen_US
dc.citation.volume17en_US
dc.citation.spage310en_US
dc.citation.epage316en_US
dc.contributor.department應用化學系zh_TW
dc.contributor.departmentDepartment of Applied Chemistryen_US
dc.identifier.wosnumberWOS:000354503600003en_US
dc.citation.woscount0en_US
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