標題: Magnetostructural coupling and multiferroic properties in the spin-frustrated system Ni1-xZnxCr2O4
作者: Chandrasekhar, K. Devi
Murthy, J. Krishna
Lin, J. -Y.
Wu, H. C.
Tseng, W. J.
Venimadhav, A.
Yang, H. D.
物理研究所
Institute of Physics
公開日期: 28-Nov-2016
摘要: The magnetic phase diagram of Ni1-xZnxCr2O4 demonstrates complex magnetic transitions for x = 0.05 with two long-range magnetic- order transitions at T-C1 = 41K and T-C2 = 17 K. A glasslike feature emerges between TC1 and TC2 with the application of a direct current (dc) magnetic field in alternating current (ac) susceptibility measurements. Dielectric measurements show a change from the conventional dielectric to a quantum-paraelectric-like behavior without anomalies near the magnetic ordering temperature in the range 0.05 <= x <= 1. The strong correlation among magnetic, dielectric, and ferroelectric properties near the structural relaxation temperatures 41 and 17 K confirms the emergence of multiferroic behavior in Ni0.95Zn0.05Cr2O4. A significant x-ray magnetic circular dichroism signal at the Ni site and ac susceptibility measurements indicate a spin-canting behavior between TC1 and TC2. The dilute doping of the non-Jahn-Teller Zn ion in the Jahn-Teller Ni site modulate the different magnetic exchange interactions of Ni and Cr, which could invoke spin-canting and multiferroic behaviors.
URI: http://dx.doi.org/10.1103/PhysRevB.94.205143
http://hdl.handle.net/11536/132804
ISSN: 2469-9950
DOI: 10.1103/PhysRevB.94.205143
期刊: PHYSICAL REVIEW B
Volume: 94
Issue: 20
起始頁: 0
結束頁: 0
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