標題: | Engineering Ultrafast Carrier Dynamics at the Graphene/GaAs Interface by Bulk Doping Level |
作者: | Yang, Jinghuan Sun, Quan Liu, Wei Zhang, Zhibin Hu, Xiaoyong Liu, Kaihui Yang, Hong Misawa, Hiroaki Gong, Qihuang 交大名義發表 National Chiao Tung University |
關鍵字: | graphene;GaAs heterostructure;photoemission electron microscopy;ultrafast carrier transfer |
公開日期: | 1-十月-2019 |
摘要: | Carrier dynamics, the most fundamental process in electronics and optoelectronics, has drawn great attentions owing to its crucial role in property engineering of materials. Exploration and regulation of carrier dynamics are essential for designing devices with specific functions and optimizing their performances. However, the lack of conventional tools with simultaneous ultrafast temporal and ultrasmall spatial resolution has impeded direct observation and manipulation of carrier dynamics at both the femtosecond and nanometer scale. In this study, the direct observation and modulation of ultrafast carrier dynamics at the graphene/gallium arsenide (GaAs) interface is achieved by tuning the doping level of bulk GaAs. This successful characterization is performed using advanced in situ photoemission electron microscopy combined with the ultrafast pump-probe technique. It is found that a change in the doping level in GaAs can change its band bending and switch the hot-carrier transfer direction at the graphene/GaAs interface with a lifetime reduction of nearly six times. This work paves the way of engineering ultrafast carrier dynamics at 2D interfaces by modifying the 3D bulk properties, and also provides a platform for fundamental studies of ultrafast physics with high spatial resolution. |
URI: | http://dx.doi.org/10.1002/adom.201900580 http://hdl.handle.net/11536/153044 |
ISSN: | 2195-1071 |
DOI: | 10.1002/adom.201900580 |
期刊: | ADVANCED OPTICAL MATERIALS |
Volume: | 7 |
Issue: | 19 |
起始頁: | 0 |
結束頁: | 0 |
顯示於類別: | 期刊論文 |